图文目录合集｜ GEE Volume 6, Issue 1

Volume 6, Issue 1

Green Energy & Environment 第六卷第一期已正式出版。

本期共收录文章17篇，其中editorial，research highlight，viewpoint和short review 各1篇，short communication和review article各2篇，research paper9篇。涉及无监督机器学习亮点评述，锂浆料电池发展前景展望，碳负载金催化剂合成氯乙烯，生物质转化乙醇，生物碱降解土壤污染物，二氧化碳催化转化以及金属有机框架的绿色应用等内容。好文多多，敬请阅读~

*封面文章：华东理工大学江浩教授团队研究论文：Confining MoS₂ nanocrystals in MOF-derived carbon for high performance lithium and potassium storage。

封底文章：佛山科学技术学院胡飞教授和华南理工大学奚红霞教授团队综述：Recent advancements in metal–organic frameworks for green applications。

图文目录

Content

 Editorial

Celebrating the 5th year of Green Energy & Environment (GEE)

Suojiang Zhang*（张锁江）

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https://doi.org/10.1016/j.gee.2021.02.007

 Research highlight

Unsupervised machine learning accelerates solid electrolyte discovery

Xu Zhang, Bin Tang, Zhen Zhou*（周震）

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https://doi.org/10.1016/j.gee.2019.12.003

Viewpoint

Lithium slurry flow cell, a promising device for the future energy storage

Lan Zhang, Xiangkun Wu, Weiwei Qian, Haitao Zhang, Suojiang Zhang*（张锁江）

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https://doi.org/10.1016/j.gee.2020.09.012

Short communications

Stabilizing supported gold catalysts in acetylene hydrochlorination by constructing an acetylene–deficient reaction phase

Bolin Wang, Yuxue Yue, Saisai Wang, Shujuan Shao, Zhi Chen, Xianhua Fang, Xiangxue Pang, Zhiyan Pan, Jia Zhao*（赵佳）, Xiaonian Li*（李小年）

We have proposed a new strategy for constructing a C₂H₂-deficient reaction phase around the active site by coating an IL film on the surface of Au(H₂O)/C, leading to great improvement in the catalytic stability of Au(H₂O)/C catalyst. Our work provides a universal method for tuning the stoichiometric balance of reactants.

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https://doi.org/10.1016/j.gee.2020.06.012

A novel hybrid digestion-gasification process integrated with membranes for efficient conversion of biomass to bio-alcohols

Xuezhong He*（何雪忠）

An innovative hybrid anaerobic digestion/chemical looping gasification process integrated with membranes was designed for production of bioalcohol used in transport sector from various feedstocks of biomass at a low environmental impact and a low cost.

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https://doi.org/10.1016/j.gee.2020.04.003

 Short review

Synthesis of 2,5-diformylfuran from renewable carbohydrates and its applications: A review

Jinhang Dai*（代金杭）

Catalytic conversion of renewable carbohydrates provides a sustainable access to value-added products. An introduction into recent developments and challenges for the production and application of 2,5-diformylfuran is highlighted herein.

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https://doi.org/10.1016/j.gee.2020.06.013

Review articles

Recent advancements in metal–organic frameworks for green applications

Chongxiong Duan, Yi Yu, Jing Xiao, Yuanyuan Li, Pengfei Yang, Fei Hu*（胡飞）, Hongxia Xi*（奚红霞）

This review summarizes the recent advances of MOFs in the fields of green applications, including carbon capture, harmful gas removal, sewage treatment, and green energy storage. The challenges and prospects of the large-scale commercialized use of MOFs in handling environmental issues are also discussed.

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https://doi.org/10.1016/j.gee.2020.04.006

The application and progress of bioelectrochemical systems (BESs) in soil remediation: A review

Tian Li¹, Ruixiang Li¹, Qixing Zhou*（周启星）

Bioelectrochemical system, as a promising technology, has been widely used in the degradation of different pollutants in different media. This paper focuses on the application of BESs in the degradation of soil pollutants.

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https://doi.org/10.1016/j.gee.2020.06.026

Research papers

Novel HBD-containing Zn (dobdc) (datz) as efficiently heterogeneous catalyst for CO₂ chemical conversion under mild conditions

Jianwen Lan, Ye Qu, Ping Xu, Jianmin Sun*（孙建敏）

Novel 3D MOF Zn (dobdc) (datz) with hydrogen bond donors (HBD) groups showed excellent catalytic performance for CO₂ conversion to cyclic carbonates under mild conditions or even room temperature, it presented high catalytic activity within consecutive six runs and was easily recycled by simple centrifugation.

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https://doi.org/10.1016/j.gee.2019.12.005

Confining MoS₂ nanocrystals in MOF-derived carbon for high performance lithium and potassium storage

Chen Hu, Kun Ma, Yanjie Hu, Aiping Chen*（陈爱平）, Petr Saha, Hao Jiang*（江浩）, Chunzhong Li

Confined synthesis tactic has been applied to realize the MoS₂ nanocrystals well-distributed into the MOF-derived porous carbon for effectively refraining their aggregation and sulfur-dissolution during electrochemical process, exhibiting greatly enhanced lithium and potassium storage performances.

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https://doi.org/10.1016/j.gee.2020.02.001

Kinetics study of CO₂ absorption in potassium carbonate solution promoted by diethylenetriamine

Rouzbeh Ramezani*, Renzo Di Felice

Reaction kinetics between CO₂ and K₂CO₃ + DETA solution were studied. The density, viscosity, reaction rate constant, reaction order, activation energy and absorption flux of CO₂ into solution were reported.

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https://doi.org/10.1016/j.gee.2019.11.004

Metallurgical pyrolysis toward Co@Nitrogen-doped carbon composite for lithium storage

Yanyan Liu, Kang Sun, Jianchun Jiang*（蒋剑春）, Wenshu Zhou, Yuan Shang, Chenxia Du, Baojun Li

Co based metal−organic frameworks are used as pyrolysis precursor to prepare nitrogen-doped carbon-Co composites possessing core-shell@sheet structure. The experimental results, combining with the theoretical calculation, demonstrate an effective metallurgical method for the construction of elemental state Li storage materials.

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https://doi.org/10.1016/j.gee.2020.03.003

The adsorption properties of NaY zeolite for separation of ethylene glycol and 1,2-butanediol: Experiment and molecular modelling

Pei Xiong, Peng He*（贺鹏）, Yixin Qu, Liguo Wang*（王利国）, Yan Cao, Shuang Xu, Jiaqiang Chen, Muhammad Ammar, Huiquan Li*（李会泉）

NaY zeolite is applied in the adsorption separation of ethylene glycol (EG) and 1,2-butanediol (1,2-BDO). The adsorption properties of NaY was studied by experiment; competition adsorption and diffusion characteristics in different adsorption regions was investigated by molecular modelling.

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https://doi.org/10.1016/j.gee.2019.12.006

Investigation the improvement of high voltage spinel LiNi_0.5Mn_1.5O₄ cathode material by anneal process for lithium ion batteries

Chao Gao, Haiping Liu*（刘海萍）, Sifu Bi, Huilin Li, Chengshuai Ma

The LiNi_0.5Mn_1.5O₄ sample treated with anneal process presents superior cycling stability compared with the initial sample. The better cycling stability is ascribed to the better electronic conductivity induced by the thin layer originated from anneal process and the more stable crystal structure.

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https://doi.org/10.1016/j.gee.2020.03.001

Hydrolysis hydrogen production mechanism of Mg10Ni10Ce alloy surface modified by SnO₂ nanotubes in different aqueous systems

Xiaojiang Hou*（侯小江）, Lu Yang, Kaiming Hou, Hongchang Shi, Lei Feng*（冯雷）, Guoquan Suo, Xiaohui Ye, Li Zhang, Yanling Yang

Simulated seawater (3.5 wt% NaCl) is proved to be an ideal medium for hydrolysis H₂ production. And SnO₂ nanotubes with unique microstructure, can accelerate the initial hydrolysis rate and enhance the final H₂ generation yield of Mg10Ni10Ce.

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https://doi.org/10.1016/j.gee.2020.05.003

Cross-polymerization between the model furans and phenolics in bio-oil with acid or alkaline catalysts

Qing Xu, Xun Hu*（胡勋）, Lijun Zhang, Kai Sun, Yuewen Shao, Zhiran Gao, Qing Liu, Chun-Zhu Li*（李春柱）

The typical furans (furfural) and phenolics (vanillin) in bio-oil interact with each other, namely cross-polymerization, which leads to changes in the functionalities, structure, morphology, and stability of the insoluble polymer.

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https://doi.org/10.1016/j.gee.2020.03.009

Understanding the molecular structure of HSW coal at atomic level: A comprehensive characterization from combined experimental and computational study

Wei Feng¹, Zhuangmei Li¹, Hongfeng Gao, Qiang Wang, Hongcun Bai*（白红存）, Ping Li*（李平）

Hongshiwan (HSW) coal are characterized by materials characterizations. Then molecular model of the coal are built with computer-aided modeling. Thus molecular structure of HSW coal have been depicted and understood at atomic level from experimental and quantum chemical approaches.

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https://doi.org/10.1016/j.gee.2020.03.013

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