庆祝农历新年，Chemical Science 审稿人推荐的中国大陆作者论文合辑

值此 2018 新春佳节，小编非常感谢大家过去一年来的支持，并祝大家在新的一年里科研工作顺利，狗年旺旺，论文足"够"多 

为庆祝中国农历新年，也为了彰显中国科学家取得的优异科研成果，英国皇家化学会旗舰期刊 Chemical Science 特别整合出中国大陆作者近两年发表的优秀论文（根据审稿人的推荐意见）合辑，范围涵盖分析科学、催化、化学生物学、材料科学、有机化学、物理化学、超分子化学等。

Chemical Science 自 2015 年起成为开放获取期刊并免收版面费。欢迎点击文末左下角“阅读原文”链接下载和阅读全文。

论文列表

排名不分先后，仅列出中国大陆单位（包括兼职）的通讯作者信息。

通讯：郑俊荣（北京大学）

Edge Article

Isotropic ordering of ions in ionic liquids on the sub-nanometer scale

Hailong Chen, Xin Chen, Jingwen Deng and Junrong Zheng

Chem. Sci., 2018, 9, 1464-1472

http://dx.doi.org/10.1039/C7SC05184K

概述 / Summary

This article investigates structures of ionic liquids.

通讯：曲大辉（华东理工）

Edge Article

One-pot synthesis of hetero[6]rotaxane bearing three different kinds of macrocycle through a self-sorting process

Si-Jia Rao, Qi Zhang, Ju Mei, Xu-Hao Ye, Chuan Gao, Qiao-Chun Wang, Da-Hui Qu* and He Tian

Chem. Sci., 2017, 8, 6777-6783

http://dx.doi.org/10.1039/C7SC03232C

概述 / Summary

A hetero[6]rotaxane bearing three different kinds of macrocycle is designed and successfully synthesized through a one-pot “click” reaction by employing a facile and efficient integrative self-sorting principle.

通讯：王炳武、郑捷、张俊龙（北京大学）

Edge Article

Enhancing the reactivity of nickel(II) in hydrogen evolution reactions (HERs) by β-hydrogenation of porphyrinoid ligands

Zhuo-Yan Wu, Teng Wang, Yin-Shan Meng, Yu Rao, Bing-Wu Wang*, Jie Zheng*, Song Gao and Jun-Long Zhang*

Chem. Sci., 2017, 8, 5953-5961

http://dx.doi.org/10.1039/C7SC02073B

概述 / Summary

β-Hydrogenation of porphyrin remarkably enhances (ca. 24 fold) the electrocatalytic HER reactivity of Ni(II) complexes.

通讯：燕红、芦昌盛（南京大学）；赵强（南京邮电）

Edge Article

Using highly emissive and environmentally sensitive o-carborane-functionalized metallophosphors to monitor mitochondrial polarity

Xiang Li, Xiao Tong, Yongheng Yin, Hong Yan*, Changsheng Lu*, Wei Huang and Qiang Zhao*

Chem. Sci., 2017, 8, 5930-5940

http://dx.doi.org/10.1039/C7SC00160F

概述 / Summary

The first o-carborane functionalized phosphorescent imaging probe of mitochondrial polarity was developed to monitor mitochondria-relevant cellular processes.

通讯：赵永席（西安交大）

Edge Article

Single copy-sensitive electrochemical assay for circulating methylated DNA in clinical samples with ultrahigh specificity based on a sequential discrimination–amplification strategy

Xuyao Wang, Feng Chen, Dexin Zhang, Yue Zhao, Jing Wei, Lihua Wang, Shiping Song, Chunhai Fan and Yongxi Zhao*

Chem. Sci., 2017, 8, 4764-4770

http://dx.doi.org/10.1039/C7SC01035D

概述 / Summary

A sequential discrimination–amplification (SEDA) electrochemical strategy was constructed for the identification of single-copy circulating methylated DNA.

通讯：姚天明、石硕（同济大学）

Edge Article

Integration of G-quadruplex and DNA-templated Ag NCs for nonarithmetic information processing

Ru-Ru Gao, Tian-Ming Yao*, Xiao-Yan Lv, Yan-Yan Zhu, Yi-Wei Zhang and Shuo Shi*

Chem. Sci., 2017, 8, 4211-4222

http://dx.doi.org/10.1039/C7SC00361G

概述 / Summary

We constructed a series of label-free and multi-output logic circuits using G-quadruplex and DNA-templated Ag NCs.

通讯：高恩庆（华东师大）；王霖（北京高压科学中心）

Edge Article

Piezochromism and hydrochromism through electron transfer: new stories for viologen materials

Qi Sui, Xiang-Ting Ren, Yu-Xiang Dai, Kai Wang, Wen-Tao Li, Teng Gong, Jia-Jia Fang, Bo Zou, En-Qing Gao* and Lin Wang*

Chem. Sci., 2017, 8, 2758-2768

http://dx.doi.org/10.1039/C6SC04579K

概述 / Summary

A pyridinium-carboxylate compound undergoes reversible color change under pressure owing to the formation of radicals via electron transfer; dehydration and hydration can also trigger electron transfer.

通讯：秦安军（华南理工）；唐本忠（港科大 / 华南理工）

Edge Article

Photoactivatable aggregation-induced emission probes for lipid droplets-specific live cell imaging

Meng Gao, Huifang Su, YuhanLin, Xia Ling, Shiwu Li, Anjun Qin* and Ben Zhong Tang*

Chem. Sci., 2017, 8, 1763-1768

http://dx.doi.org/10.1039/C6SC04842K

概述 / Summary

Photoactivatable probes for lipid droplets (LDs)-specific live-cell imaging are powerful tools for investigating their biological functions through precise spatial and temporal control.

通讯：唐本忠（港科大 / 华南理工）

Edge Article

AIE-active theranostic system: selective staining and killing of cancer cells

Chen Gui, Engui Zhao, Ryan T. K. Kwok, Anakin C. S. Leung, Jacky W. Y. Lam, Meijuan Jiang, Haiqin Deng, Yuanjing Cai, Weijie Zhang, Huifang Su and Ben Zhong Tang*

Chem. Sci., 2017, 8, 1822-1830

http://dx.doi.org/10.1039/C6SC04947H

概述 / Summary

A mitochondrion-specific AIEgen is a theranostic molecule, with the function of lighting up and killing cancer cells rather than normal cells.

通讯：俞书宏（中国科大）

Edge Article

A one-dimensional porous carbon-supported Ni/Mo2C dual catalyst for efficient water splitting

Zi-You Yu, Yu Duan, Min-Rui Gao, Chao-Chao Lang, Ya-Rong Zheng and Shu-Hong Yu*

Chem. Sci., 2017, 8, 968-973

http://dx.doi.org/10.1039/C6SC03356C

概述 / Summary

A new porous carbon-supported Ni/Mo2C composite exhibits high activity towards both the hydrogen evolution reaction and oxygen evolution reaction for overall water splitting.

通讯：危岩、吉岩（清华大学）

Edge Article

Multi-stimuli responsive and multi-functional oligoaniline-modified vitrimers

Qiaomei Chen, Xiaowen Yu, Zhiqiang Pei, Yang Yang, Yen Wei* and Yan Ji*

Chem. Sci., 2017, 8, 724-733

http://dx.doi.org/10.1039/C6SC02855A

概述 / Summary

Introducing oligoaniline into avitrimer resulted in a smart material that simultaneously responds to six different stimuli and performs six different functions.

通讯：罗三中（中科院化学所）

Edge Article

Reagent-controlled enantioselectivity switch for the asymmetric fluorination of β-ketocarbonyls by chiral primary amine catalysis

Yang'en You, Long Zhang and Sanzhong Luo*

Chem. Sci., 2017, 8, 621-626

http://dx.doi.org/10.1039/C6SC03109A

概述 / Summary

A swap of fluorination reagents led to a switch of enantioselectivity in a chiral primary amine catalyzed asymmetric α-fluorination of β-ketocarbonyls.

通讯：徐东升（北京大学）

Edge Article

Photothermal-enhanced catalysis in core-shell plasmonic hierarchical Cu₇S₄ microsphere@zeolitic imidazole framework-8

Feifan Wang, Yanjie Huang, Zhigang Chai, Min Zeng, Qi Li, Yuan Wang and Dongsheng Xu*

Chem. Sci., 2016, 7, 6887-6893

http://dx.doi.org/10.1039/C6SC03239G

概述 / Summary

A strategy to improve reaction activity via the photothermal effect of plasmonic semiconductor nanomaterials is demonstrated in a core-shell structured catalyst.

通讯：高希珂（中科院上海有机所）

Edge Article

Biazulene diimides: a new building block for organic electronic materials

Hanshen Xin, Congwu Ge, Xiaodi Yang, Honglei Gao, Xiaochun Yang and Xike Gao*

Chem. Sci., 2016, 7, 6701-6705

http://dx.doi.org/10.1039/C6SC02504H

概述 / Summary

The first class of azulene-based aromatic diimides, 2,2′-biazulene-1,1′,3,3′-tetracarboxylic diimides (BAzDIs), is presented.

通讯：李久艳（大连理工）

Edge Article

Dual n-type units including pyridine and diphenylphosphine oxide: effective design strategy of host materials for high-performance organic light-emitting diodes

Wei Li, Jiuyan Li*, Di Liu, Deli Li and Dan Zhang

Chem. Sci., 2016, 7, 6706-6714

http://dx.doi.org/10.1039/C6SC01797E

概述 / Summary

The direct linking of dual n-type units is developed to design novel host materials for improved performance of blue and green phosphorescent organic light-emitting diodes.

通讯：罗海、邵元华（北京大学）

Edge Article

Mass spectrometric snapshots for electrochemical reactions

Ran Qiu, Xin Zhang, Hai Luo* and Yuanhua Shao*

Chem. Sci., 2016, 7, 6684-6688

http://dx.doi.org/10.1039/C6SC01978A

概述 / Summary

A hybrid microelectrode can connect MS and electrochemical reactions, providing direct information on products or intermediates to identify the reaction mechanisms with easy use and low cost.

通讯：董绍俊（中科院长春应化所）

Edge Article

Self-powered fluorescence display devices based on a fast self-charging/recharging battery (Mg/Prussian blue)

Hui Zhang, You Yu, Lingling Zhang, Yiwen Zhai and Shaojun Dong*

Chem. Sci., 2016, 7, 6721-6727

http://dx.doi.org/10.1039/C6SC02347A

概述 / Summary

Here we designed and fabricated a self-powered fluorescence display device based on a fast-charging/recharging battery, composed of a Prussian blue (PB) cathode and a magnesium metal anode with a high theoretical redox potential difference.

通讯：谢浩、傅正义（武汉理工）

Edge Article

Confined-space synthesis of nanostructured anatase, directed by genetically engineered living organisms for lithium-ion batteries

Hang Ping, Hao Xie*, Mingyu Xiang, Bao-Lian Su, Yucheng Wang, Jinyong Zhang, Fan Zhang and Zhengyi Fu*

Chem. Sci., 2016, 7, 6330-6336

http://dx.doi.org/10.1039/C6SC02311H

概述 / Summary

Genetically engineered living organisms direct the synthesis of nanostructured anatase with nanoparticle, mesoporous structure and carbon coating characteristics which shows excellent lithium storage performance.

通讯：于萍、毛兰群（中科院化学所）

Edge Article

Observing single nanoparticle events at the orifice of a nanopipet

Ting Li, Xiulan He, Kailin Zhang, Kai Wang, Ping Yu* and Lanqun Mao*

Chem. Sci., 2016, 7, 6365-6368

http://dx.doi.org/10.1039/C6SC02241C

概述 / Summary

Single nanoparticle (NP) events are successfully observed at the orifice of a nanopipet by blocking the ionic current with a single NP.

通讯：王爱琴、张涛（中科院大连化物所）

Edge Article

Single-atom dispersed Co–N–C catalyst: structure identification and performance for hydrogenative coupling of nitroarenes

Wengang Liu, Leilei Zhang, Wensheng Yan, Xiaoyan Liu, Xiaofeng Yang, Shu Miao, Wentao Wang, Aiqin Wang* and Tao Zhang*

Chem. Sci., 2016, 7, 5758-5764

http://dx.doi.org/10.1039/C6SC02105K

概述 / Summary

The single-atom Co–N–C catalyst with the structure of CoN₄C₈-1-2O₂ shows excellent performance for the chemoselective hydrogenation of nitroarenes to produce azo compounds under mild reaction conditions.

通讯：裴坚（北京大学）

Edge Article

Embedding electron-deficient nitrogen atoms in polymer backbone towards high performance n-type polymer field-effect transistors

Ya-Zhong Dai, Na Ai, Yang Lu, Yu-Qing Zheng, Jin-Hu Dou, Ke Shi, Ting Lei, Jie-Yu Wang and Jian Pei*

Chem. Sci., 2016, 7, 5753-5757

http://dx.doi.org/10.1039/C6SC01380E

概述 / Summary

The low LUMO level and the conformation-locked planar backbone provide polymer AzaBDOPV-2T with electron mobilities over 3.22 cm2 V−1 s−1 tested in air.

通讯：唐本忠（港科大 / 华南理工）

Edge Article

Luminescent photonic crystals with multi-functionality and tunability

Hong Wang, Xinggui Gu, Rongrong Hu, Jacky W. Y. Lam, Deqing Zhang and Ben Zhong Tang*

Chem. Sci., 2016, 7, 5692-5698

http://dx.doi.org/10.1039/C6SC01703G

概述 / Summary

We develop a general method to incorporate aggregation-induced emission luminogens into photonic crystals (PCs) and the resulting luminescent PCs display diverse structural colors in response to water stimulation.

通讯：洪茂椿、陈学元（中科院福建物构所）

Edge Article

In vitro upconverting/downshifting luminescent detection of tumor markers based on Eu³⁺-activated core–shell–shell lanthanide nanoprobes

Yongsheng Liu, Shanyong Zhou, Zhu Zhuo, Renfu Li, Zhuo Chen, Maochun Hong* and Xueyuan Chen*

Chem. Sci., 2016, 7, 5013-5019

http://dx.doi.org/10.1039/C6SC01195K

概述 / Summary

We demonstrate the successful use of Eu³⁺-activated core–shell–shell nanoprobes for in vitro upconverting/downshifting luminescent detection of a cancer biomarker of alpha-fetoprotein.

通讯：王炳武、高松（北京大学）

Edge Article

Thermostability and photoluminescence of Dy(III) single-molecule magnets under a magnetic field

Ye Bi, Cheng Chen, Yi-Fang Zhao, Yi-Quan Zhang, Shang-Da Jiang, Bing-Wu Wang*, Jun-Bo Han, Jun-Liang Sun, Zu-Qiang Bian, Zhe-Ming Wang and Song Gao*

Chem. Sci., 2016, 7, 5020-5031

http://dx.doi.org/10.1039/C6SC01157H

概述 / Summary

A series of promising multifunctional lanthanide single-molecule magnets (SMMs). Lanthanide luminescence under a pulsed magnetic field for SMMs is examined for the first time.

通讯：夏清华（湖北大学）

Edge Article

One-pot rota-crystallized hollownest-structured Ti–zeolite: a calcination-free and recyclable catalytic material

Dan Zhou, Tianjun Zhang, Qinghua Xia*, Yarong Zhao, Kexin Lv, Xinhuan Lu and Renfeng Nie

Chem. Sci., 2016, 7, 4966-4972

http://dx.doi.org/10.1039/C6SC01735E

概述 / Summary

A hydrothermal rota-crystallization method is developed for the one-step synthesis of ahollownest-structured zeolite precursor with the shell composed of autogenously-intergrown MWW nanosheet crystals containing a large number of stacking-pores without any porogen or hard scaffold.

通讯：孟鸿（北京大学深圳研究生院）；陈红征（浙江大学）；黄维（南京工业大学先进材料研究院）

Edge Article

Effects of heteroatom substitution in spiro-bifluorene hole transport materials

Zhao Hu, Weifei Fu, Lijia Yan, Jingsheng Miao, Hongtao Yu, Yaowu He, Osamu Goto, Hong Meng*, Hongzheng Chen* and Wei Huang*

Chem. Sci., 2016, 7, 5007-5012

http://dx.doi.org/10.1039/C6SC00973E

概述 / Summary

By introducing the heteroatom into the benchmark hole transport material Spiro-MeOTAD, the energy level of hole transport materials can be tuned.

通讯：李景虹（清华大学）

Edge Article

Cas9 cleavage assay for pre-screening of sgRNAs using nicking triggered isothermal amplification

Kaixiang Zhang, Ruijie Deng, Yue Li, Ling Zhang and Jinghong Li*

Chem. Sci., 2016, 7, 4951-4957

http://dx.doi.org/10.1039/C6SC01355D

概述 / Summary

A novel Cas9 cleavage assay was developed for quantitative evaluation of Cas9 cleavage efficiency and pre-screening of sgRNA to achieve highly specific and highly efficient CRISPR/Cas9 genome editing.

通讯：刘成辉、李正平（陕西师大）

Edge Article

Ultrasensitive detection of telomerase activity in a single cell using stem-loop primer-mediated exponential amplification (SPEA) with near zero nonspecific signal

Honghong Wang, Hui Wang, Chenghui Liu*, Xinrui Duan and Zhengping Li*

Chem. Sci., 2016, 7, 4945-4950

http://dx.doi.org/10.1039/C6SC00802J

概述 / Summary

A SPEA strategy is developed for the detection of telomerase activity in a single cell with a near zero nonspecific signal.

通讯：唐建斌（浙江大学）；郭志前、朱为宏（华东理工）

Edge Article

Dual-channel NIR activatable theranostic prodrug for in vivo spatiotemporal tracking thiol-triggered chemotherapy

Mingzhou Ye, Xiaohang Wang, Jianbin Tang*, Zhiqian Guo*, Youqing Shen, He Tian and Wei-Hong Zhu*

Chem. Sci., 2016, 7, 4958-4965

http://dx.doi.org/10.1039/C6SC00970K

概述 / Summary

Real-time tracking of where, when, and how prodrugs are established. A novel theranostic prodrug based on the disulfide linkage with two distinct switchable near-infrared (NIR) fluorescence can precisely extract the prodrug release profile in vivo through dual-channel fluorescent imaging for the first time.

通讯：张长生（中科院南海海洋所）

Edge Article

Flavoenzyme CrmK-mediated substrate recycling in caerulomycin biosynthesis

Yiguang Zhu, Marie-Ève Picard, Qingbo Zhang, Julie Barma, Xavier Murphy Després, Xiangui Mei, Liping Zhang, Jean-Baptiste Duvignaud, Manon Couture, Weiming Zhu, Rong Shi* and Changsheng Zhang*

Chem. Sci., 2016, 7, 4867-4874

http://dx.doi.org/10.1039/C6SC00771F

概述 / Summary

Biochemical and structural investigations into the flavoenzyme CrmK reveal a substrate recycling/salvaging mechanism in caerulomycin biosynthesis.

通讯：谢建华（南开大学）

Edge Article

Divergent enantioselective synthesis of hapalindole-type alkaloids using catalytic asymmetric hydrogenation of a ketone to construct the chiral core structure

Yang Liu, Li-Jie Cheng, Hai-Tao Yue, Wen Che, Jian-Hua Xie* and Qi-Lin Zhou

Chem. Sci., 2016, 7, 4725-4729

http://dx.doi.org/10.1039/C6SC00686H

概述 / Summary

A divergent enantioselective approach to hapalindole-type alkaloids featuring a ruthenium-catalyzed asymmetric hydrogenation and a switchable sequence of methylation and acetylation/aldol reaction is described.

通讯：朱本占（中科院生态环境中心）

Edge Article

Delivering the cell-impermeable DNA ‘light-switching’ Ru(II) complexes preferentially into live-cell nucleus via an unprecedented ion-pairing method

Ben-Zhan Zhu*, Xi-Juan Chao, Chun-Hua Huang and Yan Li

Chem. Sci., 2016, 7, 4016-4023

http://dx.doi.org/10.1039/C5SC03796D

概述 / Summary

The cell-impermeable DNA ‘light-switching’ Ru(II) complexes can be delivered into live-cell nucleus by forming lipophilic Yin–Yang ion-pairs with hydrophobic weak-acids.

通讯：唐波（山东师大）

Edge Article

Anuclear targeted dual-photosensitizer for drug-resistant cancer therapy with NIR activated multiple ROS

Zhengze Yu, Wei Pan, Na Li and Bo Tang*

Chem. Sci., 2016, 7, 4237-4244

http://dx.doi.org/10.1039/C6SC00737F

概述 / Summary

Anuclear targeted dual-photosensitizer was developed for photodynamic therapy against multidrug resistant cancer. Multiple reactive oxygen species (ROS) could be generated in the nucleus to directly break DNA double strands with a single 980 nm NIR laser irradiation, regardless of drug resistance.

通讯：俞书宏（中国科大）

Edge Article

A general chemical transformation route to two-dimensional mesoporous metal selenide nanomaterials by acidification of a ZnSe–amine lamellar hybrid at room temperature

Zeng-Wen Hu, Liang Xu, Yuan Yang, Hong-Bin Yao, Hong-Wu Zhu, Bi-Cheng Hu and Shu-Hong Yu*

Chem. Sci., 2016, 7, 4276-4283

http://dx.doi.org/10.1039/C6SC00674D

概述 / Summary

A family of mesoporous nanosheets of metal selenides can be synthesized using an intermediate precursor so-called “red Se remaining Zn” (RSRZ), which is generated by acidification ofinorganic–organichybrid ZnSe(DETA)0.5nanosheets.

通讯：李敬、汪尔康（中科院长春应化所）

Edge Article

Noble-metal-free Co₃S₄–S/G porous hybrids as an efficient electrocatalyst for oxygen reduction reaction

Wenling Gu, Liuyong Hu, Wei Hong, Xiaofang Jia, Jing Li* and Erkang Wang*

Chem. Sci., 2016, 7, 4167-4173

http://dx.doi.org/10.1039/C6SC00357E

概述 / Summary

A high-efficiency noble-metal-free oxygen reduction reaction (ORR) catalyst was obtained based on the pyrolysis of the inexpensive precursor cobalt dithiolene (an S₄-chelate complex) on simultaneously reduced graphene oxide (GO) as a support matrix.

通讯：王柯敏（湖南大学）

Edge Article

Fluorescence resonance energy transfer-based hybridization chain reaction for in situ visualization of tumor-related mRNA

Jin Huang, He Wang, Xiaohai Yang, Ke Quan, Yanjing Yang, Le Ying, Nuli Xie, Min Ou and Kemin Wang*

Chem. Sci., 2016, 7, 3829-3835

http://dx.doi.org/10.1039/C6SC00377J

概述 / Summary

The ability to visualize tumor-related mRNA in situ in single cells would distinguish whether they are cancer cells or normal cells, which holds great promise for cancer diagnosis at an early stage.

通讯：李激扬、于吉红（吉林大学）

Edge Article

Carbogenic nanodots derived from organo-templated zeolites with modulated full-color luminescence

Ying Mu, Ning Wang, Zaicheng Sun, Jing Wang, Jiyang Li* and Jihong Yu*

Chem. Sci., 2016, 7, 3564-3568

http://dx.doi.org/10.1039/C6SC00085A

概述 / Summary

Dual modulated luminescence of carbogenic nanodots derived from zeolites has been acquired by controlling the concentration and pH value of CND aqueous dispersions.

通讯：许乃寒（清华大学深圳研究生院）；李子刚（北京大学深圳研究生院）

Edge Article

Stapling of unprotected helical peptides via photo-induced intramolecular thiol–yne hydrothiolation

Yuan Tian, Jingxu Li, Hui Zhao, Xiangze Zeng, Dongyuan Wang, Qisong Liu, Xiaogang Niu, Xuhui Huang, NaihanXu* and Zigang Li*

Chem. Sci., 2016, 7, 3325-3330

http://dx.doi.org/10.1039/C6SC00106H

概述 / Summary

A one component intramolecular thiol–yne macrocyclization is achieved upon UV irradiation to constrain short unprotected peptides into a helical conformation, providing rapid access to stapled peptides with satisfying functional group tolerance.

通讯：李根喜（南京大学）

Edge Article

Improvement of enzyme-linked immunosorbent assay for the multicolor detection of biomarkers

Chao Li, Yucai Yang, Dan Wu, Tianqi Li, Yongmei Yin and Genxi Li*

Chem. Sci., 2016, 7, 3011-3016

http://dx.doi.org/10.1039/C5SC04256A

概述 / Summary

An activatable graphene-based nanoprobe is used to develop a multicolor immunosorbent assay for the detection of tumor protein biomarkers.

通讯：王心晨（福州大学）

Edge Article

Overall water splitting by Pt/g-C₃N₄ photocatalysts without using sacrificial agents

Guigang Zhang, Zhi-An Lan, Lihua Lin, Sen Lin and Xinchen Wang*

Chem. Sci., 2016, 7, 3062-3066

http://dx.doi.org/10.1039/C5SC04572J

概述 / Summary

Direct splitting of pure water into H₂ and O₂ in a stoichiometric molar ratio of 2:1 by conjugated polymers via a 4-electron pathway was established for the first time, as demonstrated here using a g-C₃N₄ polymer and redox co-catalysts of Pt and Co species.

通讯：陈学元（中科院福建物构所）

Edge Article

Sub-5 nm lanthanide-doped lutetium oxyfluoride nanoprobes for ultrasensitive detection of prostate specific antigen

Jin Xu, Shanyong Zhou, Datao Tu, Wei Zheng, Ping Huang, Renfu Li, Zhuo Chen, Mingdong Huang and Xueyuan Chen*

Chem. Sci., 2016, 7, 2572-2578

http://dx.doi.org/10.1039/C5SC04599A

概述 / Summary

We demonstrate the successful use of sub-5 nm Lu₆O₅F₈:Eu³⁺ nano-bioprobes for the ultrasensitive detection of prostate specific antigen in patient serum samples with a limit of detection of 0.52 pg mL−1.

通讯：曲大辉（华东理工）

Edge Article

One-pot synthesis of a [c2]daisy-chain-containing hetero[4]rotaxane via a self-sorting strategy

Xin Fu, Qi Zhang, Si-Jia Rao, Da-Hui Qu* and He Tian

Chem. Sci., 2016, 7, 1696-1701

http://dx.doi.org/10.1039/C5SC04844C

概述 / Summary

Here we demonstrated a facile and efficient one-pot synthesis of a [c2]daisy-chain-containing hetero[4]rotaxane via a self-sorting strategy.

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