图文目录|GEE Volume 6, Issue 6
Volume 6, Issue 6
Green Energy & Environment第六卷第六期已正式出版。本期共收录文章16篇,其中research highlight 1篇,review article 2篇,research paper 13篇。部分文章中文解读已推送,点击中文标题即可阅读。其他文章中文解读将在近期推送,敬请关注~
*封面文章:浙江工业大学王建国教授团队研究论文——Building highly active hybrid double–atom sites in C2N for enhanced electrocatalytic hydrogen peroxide synthesis。
封底文章:中北大学焦纬洲教授课题组研究论文——Degradation of nitrobenzene-containing wastewater by sequential nanoscale zero valent iron-persulfate process。
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Research highlight
Long-cycling and dendrite-free lithium metal anodes via salt chemistry
Sainan Liu, Wenchao Zhang*(张文超)
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https://doi.org/10.1016/j.gee.2021.02.009
02Review articles
Boron based hypergolic ionic liquids: A review
Zhenyu Zhang, Zirui Zhao, Binshen Wang*(王滨燊), Jiaheng Zhang*(张嘉恒)
Boron-based hypergolic ionic liquids (HILs) and their derivatives are discussed herein, which is a promising family for potential bipropellant systems. Specially, physicochemical properties and ignition performance of these green fuel are highlighted.
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https://doi.org/10.1016/j.gee.2020.12.002
Multidimensional (0D-3D) functional nanocarbon: Promising material to strengthen the photocatalytic activity of graphitic carbon nitride
Bin He, Mi Feng, Xinyan Chen, Jian Sun*(孙剑)
Strategies on employing multidimensional (0D∼3D) functional nanocarbon materials as modifiers to strengthen visible-light photocatalytic activity of g-C3N4 were reviewed. And a nichetargeting outlook on the major challenges, and opportunities for high-powered carbon/g-C3N4 composites were also proposed.
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多维度功能化纳米碳材料—光催化的“加油站”
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https://doi.org/10.1016/j.gee.2020.07.011
03Research papers
Building highly active hybrid double–atom sites in C2N for enhanced electrocatalytic hydrogen peroxide synthesis
Yongyong Cao, Jinyan Zhao, Xing Zhong, Guilin Zhuang, Shengwei Deng, Zhongzhe Wei, Zihao Yao, Jianguo Wang*(王建国)
RuCu@C2N (Rubine) and PdCu@C2N (Emerald) for the synthesis of H2O2 via oxygen reduction reaction are designed. Emerald shows a higher catalytic performance for electrocatalytic H2O2 synthesis with lower overpotential and dynamic energy barrier compared with Rubine.
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杂双原子催化剂高效电催化合成双氧水
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https://doi.org/10.1016/j.gee.2020.12.006
Continuous synthesis of few-layer MoS2 with highly electrocatalytic hydrogen evolution
Meng Shao1, Peican Wang1, Yimeng Wang, Baoguo Wang*(王保国), Yundong Wang, Jianhong Xu*(徐建鸿)
A continuous micro-reaction approach with high heat and mass transfer rates to synthesize few-layer MoS2 nanoplates with abundant active sites was developed. The defective MoS2 ultrathin nanoplates exhibit excellent HER performance.
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少层二硫化钼纳米片的连续可控制备与高效电催化析氢性能
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https://doi.org/10.1016/j.gee.2020.04.008
Boosting oxygen evolution reactivity by modulating electronic structure and honeycomb-like architecture in Ni2P/N,P-codoped carbon hybrids
Menglei Yuan, Yu Sun, Yong Yang, Jingxian Zhang, Sobia Dipazir, Tongkun Zhao, Shuwei Li, Yongbing Xie, He Zhao, Zhanjun Liu, Guangjin Zhang*(张光晋)
In this work, for the first time, we propose synergistic strategy that couples electronic structure and honeycomb-like architectures achieve a low-overpotential Ni2P/N,P-codoped carbon hybrids for efficient OER.
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https://doi.org/10.1016/j.gee.2020.07.012
Efficient hydrogen production through the chemical looping redox cycle of YSZ supported iron oxides
Li Ma1, Yu Qiu1, Min Li, Dongxu Cui, Shuai Zhang, Dewang Zeng*(曾德望), Rui Xiao*(肖睿)
The yttria-stabilized zirconia supported Fe2O3 showed efficient hydrogen production in the chemical looping water splitting process. The support effect provides a promising route for the modification of oxygen carrier materials.
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https://doi.org/10.1016/j.gee.2020.06.023
Zeolite-templated carbons as effective sorbents to remove methylsiloxanes and derivatives: A computational screening
Shiru Lin1, Kaitlyn A. Jacoby1, Jinxing Gu, Dariana R. Vega-Santander, Arturo J. Hernández-Maldonado*, Zhongfang Chen*(陈中方)
By Grand Canonical Monte Carlo simulations, we explored the potentials of the recently proposed 68 stable zeolite-templated carbons (ZTCs) as sorbents to remove methylsiloxanes and derivatives. Four ZTCs, namely ISV, FAU1, FAU3, and H8326836, were identified with better adsorption performance than activated carbons, and ISV is expected to perform the best.
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https://doi.org/10.1016/j.gee.2020.07.007
Novel montmorillonite-sulfur composite for enhancement of selective adsorption toward cesium
Shanqing Chen, Jiayin Hu*(胡佳音), Guoliang Mi, Yafei Guo, Tianlong Deng*(邓天龙)
Novel montmorillonite-sulfur composite was developed for the efficient and selective removal of cesium from complicated wastewater containing various competing ions.
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https://doi.org/10.1016/j.gee.2020.07.016
Assisting effect of Al2O3 on MnOx for NO catalytic oxidation
Denghui Wang*(王登辉), Hui Li, Qi Yao, Shien Hui, Yanqing Niu
Efficient catalysts for NO oxidation were prepared using MnOx as active compound, with TiO2 or Al2O3 as support. Performance of the catalysts followed as Mn0.4/Al > Mn0.2/Al > Mn0.4/Ti > Mn0.2/Ti > MnOx > Al2O3 on the whole, indicating the effective assisting influence of Al2O3 on MnOx for NO catalytic oxidation.
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https://doi.org/10.1016/j.gee.2020.07.005
Degradation of nitrobenzene-containing wastewater by sequential nanoscale zero valent iron-persulfate process
Jingjuan Qian, Weizhou Jiao*(焦纬洲), Youzhi Liu
NZVI was prepared by IS-RPB, and sequential NZVI-Na2S2O8 process was first proposed to degrade nitrobenzene-containing wastewater. The degradation mechanism was studied by EPR and radical capture experiments, and degradation pathway was studied by GC–MS.
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超重力强化纳米零价铁-过硫酸盐连续运行体系降解含硝基苯废水
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https://doi.org/10.1016/j.gee.2020.07.018
Ternary blend strategy in benzotriazole-based organic photovoltaics for indoor application
Yinglong Bai, Runnan Yu, Yiming Bai, Erjun Zhou*(周二军), Tasawar Hayat, Ahmed Alsaedi, Zhan'ao Tan*(谭占鳌)
Benzotriazole-based polymer donor J52-F, chlorinated polymer donor PM7 and A2-A1-D-A1-A2-structured acceptor BTA3 are used to construct ternary OPVs for indoor light applications. Benefitting from the introduction of PM7 as the third component in J52-F:BTA3-based blend, a gratifying PCE of 20.04% with a high VOC of 1.00 V has been achieved under the test conditions with an illumination of 300 lx from an LED lighting source with a color temperature of 3000 K.
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https://doi.org/10.1016/j.gee.2020.07.017
Controllable synthesis of nitrogen-doped porous carbon from metal-polluted miscanthus waste boosting for supercapacitors
Zuo Chen, Man Zhang, Yuchen Wang, Zhiyu Yang, Di Hu, Yetao Tang, Kai Yan*(严凯)
In this study, we fabricated nitrogen-doped nanoporous carbon with large specific area and good conductivity from metal-polluted miscanthus wastes. Furthermore, the symmetric supercapacitor assembled by the synthesized porous carbon achieved remarkable electrochemical performance.
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https://doi.org/10.1016/j.gee.2020.07.015
Photoreduction of CO2 in the presence of CH4 over g-C3N4 modified with TiO2 nanoparticles at room temperature
Ming Chen, Jiachen Wu, Chongchong Lu, Xiao Luo*(罗潇), Yangqiang Huang*, Bo Jin, Hongxia Gao, Xiaowen Zhang, Morris Argyle, Zhiwu Liang*(梁志武)
CO2 and CH4 are possible alternative energy sources. In this work, the noble-metal-free TNP-CN photocatalyst was used to convert them into value added chemicals, such as H2, CO, C2H6, C2H4 and surface acetate.
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https://doi.org/10.1016/j.gee.2020.07.001
Novel magnetic carbon supported molybdenum disulfide catalyst and its application in residue upgrading
Xiangyang Zhu, Dong Qiao, Liangrong Yang*(杨良嵘), Qinling Bi, Huifang Xing, Shan Ni, Menglei Yuan, Huizhou Liu*(刘会洲), Luhai Wang, An Ma
In this work, for the first time, we report the magnetically retrievable Fe3O4/C–MoS2 catalysts by a synergistic strategy that achieves enhanced hydrocracking performance for the actual heavy oil upgrading.
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https://doi.org/10.1016/j.gee.2020.06.025
Synthesis of HTLcs modified by K3PO4 for side chain alkylation of toluene with methanol
Chunyao Hao1, Yueli Wen1, Bin Wang*(王斌), Faraz Ahmad, Yuhua Liu, Huijun Li, Wei Huang*(黄伟)
The addition of K3PO4 could adjust the acid-base site distribution and significantly improve the catalytic activity of calcined hydrotalcite catalysts for side chain alkylation of toluene with methanol, where the highest selectivities of styrene and ethylbenzene were 39.25% and 40.68%, respectively.
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https://doi.org/10.1016/j.gee.2020.06.007
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