【科学综述】The rise of two-dimensional MoS2 for catalysis

The rise of two-dimensional MoS₂ for catalysis

Jun Mao (毛军)^1,2, Yong Wang (王勇)^1,2 , 

Zhilong Zheng (郑智龙) ^1,2, Dehui Deng (邓德会) ^1,2,†

¹State Key Laboratory of Physical Chemistry of  Solid Surfaces, Collaborative Innovation Center of Chemistry for Energy Materials (iChEM), College of  Chemistry and Chemical Engineering, Xiamen University, Xiamen 361005, China

²State Key Laboratory of  Catalysis, Collaborative Innovation Center of Chemistry for Energy Materials (iChEM), Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian 116023, China

Corresponding author. E-mail: ^†[e-mail]

Abstract:
Two-dimensional (2D) MoS₂ is used as acatalyst or support and has received increased research interest because of itssuperior structural and electronic properties compared with those of bulk structures. In this article, we illustrate the active sites of 2D MoS₂ and various strategies for enhancing its intrinsic catalytic activity. The recent advancesin the use of 2D MoS₂-based materials for applications such as thermocatalysis, electrocatalysis, and photocatalysis are discussed. We also discuss the future opportunities and challenges for 2D MoS₂-based materials, in both fundamental research and industrial applications.

Contents:

1 Introduction

2 Recognition of active sites

3 Application

3.1 Thermocatalysis

3.2 Electrocatalysis

3.3 Photocatalysis

3.3.1 Photocatalytic water splitting

3.3.2 Other reactions

4 Conclusions and perspectives 

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