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《中国科学:材料科学》2023年第4期

中国科学材料 中国科学材料 2023-07-03


Cover Story 

Electrochemical conversion of CO2 into value-added chemicals and fuels is of great importance to relieve the growing CO2 emission and achieve the carbon neutrality. Heterojunction catalysts can boost the electrochemical CO2 reduction reaction (CO2RR) by facilitating the charge transfer, but their rational construction still remains a great challenge. Liu and coworkers fabricated a Bi2O2CO3/ZnO heterojunction electrocatalyst by a hexadecyl trimethyl ammonium bromide-templated hydrothermal method, achieving the enhanced CO2-to-formate conversion efficiency and outstanding stability than single components. Electrochemical test combined with spectral analysis revealed that the interface charge transfer and produced compressive stress between the heterostructure synergistically contribute to the enhancement of CO2RR performance (see the article on page 1398).


REVIEW

Semiconductor nanomaterial-based polarized light emission: From materials to light emitting diodes

基于半导体纳米材料的偏振光发射:从材料到发光二极管

Jinlei Wu, Guoqiang Fang, Yongliang Zhang, Nandita Biswas, Yanan Ji, Wen Xu, Bin Dong (董斌), Ning Liu (刘宁)

Sci China Mater, 2023, 66(4): 1257–1282



REVIEW

3D printing metamaterials for highly efficient electromagnetic wave absorption

用于高效电磁波吸收的3D打印超材料

Rui Zhou, Zhen Yu, Zhenzhen Wu, Chang Qu, Yan Song, Ruizhe Xing, Jie Kong (孔杰)

Sci China Mater, 2023, 66(4): 1283–1312



ARTICLE

Orientation-controlled mesoporous PbI2 scaffold for 22.7% perovskite solar cells

定向控制介孔PbI2支架制备效率达22.7%的钙钛矿太阳能电池

Dejun Huang, Qianyu Liu, Zhu Ma (马柱), Yanlin Li, Guangyuan Yan, Shanyue Hou, Zhuowei Du, Junbo Yang, Yi Chen, Shufang Tang, Hengyu Zhou, Yan Xiang, Wenfeng Zhang, Yuelong Huang (黄跃龙), Yaohua Mai (麦耀华) 

Sci China Mater, 2023, 66(4): 1313–1322



ARTICLE

Reconstructing the amorphous and defective surface for efficient and stable perovskite solar cells

高效稳定钙钛矿太阳能电池中非晶和缺陷表面的重构

Jiangsheng Xie (谢江生), Shenghe Zhao, Pengjie Hang, Tian Chen, Bin Wen, Qixin Yin, Shichen Wei, Shengcai Zhu, Xuegong Yu, Minchao Qin, Xinhui Lu, Keyou Yan (严克友), Jianbin Xu (许建斌)Pingqi Gao (高平奇)

Sci China Mater, 2023, 66(4): 1323–1331



ARTICLE

Ultrathin thiol-ene crosslinked polymeric electrolyte for solid-state and high-performance lithium metal batteries

超薄烯-巯交联聚合物电解质及其固态高性能锂金属电池

Zhifeng Li, Tianyi Wang, Lei Zhong (钟雷), Min Xiao, Dongmei Han, Shuanjin Wang, Shichao Zhang, Sheng Huang, Yuezhong Meng (孟跃中)

Sci China Mater, 2023, 66(4): 1332–1340



ARTICLE

Metal sulfide heterojunction with tunable interfacial electronic structure as an efficient catalyst for lithium-oxygen batteries

具有可调界面电子结构的金属硫化物异质结构作为锂-氧气电池的高效催化剂

Guilei Tian, Longfei Ren, Haoyang Xu, Ting Zeng, Xinxiang Wang, Xiaojuan Wen, Dayue Du, Yu Yan, Sheng Liu, Chaozhu Shu (舒朝著)

Sci China Mater, 2023, 66(4): 1341–1351



ARTICLE

Boosting the interlayer-confined nitrate reduction reaction by in situ electrochemical potassium ion intercalation

原位电化学钾离子插层促进层间限域的硝酸盐还原制氨反应

Mengqiu Xu, Ye Zhang, Haiqiao Zhou, Xiaoyu Li, Yuhu Zhou, Xudong Xu, Gan Jia, Genping Zhu, Fangfang Wu (毋芳芳), Peng Gao (高鹏)Wei Ye (叶伟)

Sci China Mater, 2023, 66(4): 1352–1361



ARTICLE

Space-confined ultrafine Co4N nanodots within an N-doped carbon framework on carbon cloth for highly efficient universal pH overall water splitting

空间限域策略合成碳布负载超小Co4N纳米点复合氮掺杂碳用于高效的宽pH全解水

Deliang Zhang, Changhong Sun, Dongzheng Liu, Caixia Song (宋彩霞)Debao Wang  (王德宝)

Sci China Mater, 2023, 66(4): 1362–1372



ARTICLE

Engineering metal-organic framework nanosheets with electronically modulated in-plane heterojunctions for robust high-current-density water splitting

具有电子调制平面异质结的金属有机骨架纳米片用于高电流密度全解水

Sheng Zhao, Liming Deng, Yixing Xiong, Feng Hu, Lijie Yin, Deshuang Yu, LinLin Li, Shengjie Peng (彭生杰)

Sci China Mater, 2023, 66(4): 1373–1382



ARTICLE

Amorphous versus crystalline CoSx anchored on CNTs as heterostructured electrocatalysts toward hydrogen evolution reaction

非晶态与晶态硫化钴/碳纳米管异质结用于高效电催化析氢

Changgen Cheng, Weidong Ao, Huijun Ren, Zhishuai Fan, Tingting Xu, Lei Dai (代磊), Peiqun Yin  (尹培群)

Sci China Mater, 2023, 66(4): 1383–1388



ARTICLE

Dual Pt–Ni atoms dispersed on N-doped carbon nanostructure with novel (NiPt)-N4C2 configurations for synergistic electrocatalytic hydrogen evolution reaction

铂-镍双原子分散在具有新型(NiPt)-N4C2构型的氮掺杂碳纳米结构上用于协同电催化析氢反应

Yumin Da, Zhangliu Tian, Rui Jiang, Yuan Liu, Xu Lian, Shibo Xi, Yi Shi, Yongping Wang, Haotian Lu, Baihua Cui, Jinfeng Zhang, Xiaopeng Han (韩晓鹏), Wei Chen (陈伟), Wenbin Hu (胡文彬)

Sci China Mater, 2023, 66(4): 1389–1397



ARTICLE

Lattice strain and interfacial engineering of a Bi-based electrocatalyst for highly selective CO2 electroreduction to formate

晶格应变和异质界面工程协同促进铋基催化剂高效电催化CO2还原生成甲酸

Xiaoqian Wei, Zijian Li, Haeseong Jang, Min Gyu Kim, Qing Qin (秦清), Xien Liu (刘希恩)

Sci China Mater, 2023, 66(4): 1398–1406



ARTICLE

Porous nanosheet composite with multi-type active centers as an efficient and stable oxygen electrocatalyst in alkaline and acid conditions 

碱性和酸性条件下均稳定的高效氧电催化剂:具有多活性中心的多孔纳米片复合材料

Yannan Xia, Yi Cheng, Rui Wang, Zihan Meng, Quentin Meyer, Chuan Zhao, Haining Zhang, Ren Luo, Yang Li, Haolin Tang (唐浩林)

Sci China Mater, 2023, 66(4): 1407–1416



ARTICLE

Size-engineered noble metal nanoclusters synthesized by impregnation for size-dependent catalysis

浸渍法制备尺寸均一可调的贵金属纳米团簇及其尺寸依赖的催化性质

Zhibin Wen, Shumeng Zhang, Zhaojun Liu, Zhixue Zhang, Zhun Qiao, Kai Liu, Chuanbo Gao (高传博)

Sci China Mater, 2023, 66(4): 1417–1426



ARTICLE

Electrochemical-leaching route for the size-controllable synthesis of copper-based oxygen reduction reaction catalysts: From nanoparticles to atomic clusters and single atoms

电化学溶出法尺寸可控合成铜基氧还原反应催化剂:从纳米粒子到原子团簇和单原子

Rui Li, Jingsong Xu (徐劲松), Qingkai Zhao, Xiayan Yan, Jingwen Ba, Yaqi Song, Rongguang Zeng, Qifa Pan, Tao Tang, Wenhua Luo

Sci China Mater, 2023, 66(4): 1427–1434



ARTICLE

Mannitol and acidity co-tuned synthesis of oxygen-vacancy-modified bismuth molybdate nanorods for efficient photocatalytic nitrogen reduction to ammonia

甘露醇与酸碱度协同调控氧空位修饰钼酸铋纳米棒的合成及其高效光催化固氮活性

Guoan Wang, Quanhua Deng (邓全花), Haiping Li  (李海平), Wanguo Hou

Sci China Mater, 2023, 66(4): 1435–1446



ARTICLE

Creation of an internal electric field in SnO2@ZnS-ZnSn(OH)6 dual-type-II heterojunctions for efficient NO photo-oxidation

双II型SnO2@ZnS-ZnSn(OH)6异质结构建内部电场用 于高效光催化NO氧化去除

Bangfu Chen, Ping Ouyang, Yuhan Li (李宇涵), Youyu Duan  (段有雨), Kangle Lv, Sónia A.C. Carabineiro, Fan Dong

Sci China Mater, 2023, 66(4): 1447–1459



ARTICLE

rGO spatially confined growth of ultrathin In2S3 nanosheets for construction of efficient quasi-one-dimensional Sb2Se3-based heterojunction photocathodes

rGO空间限域生长超薄In2S3纳米片用于构建高效准一维Sb2Se3基异质结光阴极

Yufei Cheng, Qian Sun, Qiujie Li, Wenwan Zhang, Enzhou Liu, Jun Fan, Haijiao Xie, Hui Miao (苗慧), Xiaoyun Hu (胡晓云)

Sci China Mater, 2023, 66(4): 1460–1470



ARTICLE

Construction of Au/Cu hierarchically organized particles with dual-functional enzyme-like activity具有双功能酶活性的Au/Cu多级组装颗粒的构建Qing Li, Jiaxing Zhang, Yuefei Wang (王跃飞), Jiwei Min, Yuhe Shen, Wei Liu, Xuefeng Liu, Rongxin Su, Wei Qi (齐崴)Sci China Mater, 2023, 66(4): 1471–1483



ARTICLE

Three-dimensional Dirac semimetal (Cd1-xZnx)3As2/Sb2Se3 back-to-back heterojunction for fast-response broadband photodetector with ultrahigh signal-to-noise ratio

3D狄拉克半金属(Cd1-xZnx)3As2/Sb2Se3背对背异质结用于超高信噪比的高速宽光谱光电探测器

Xingchao Zhang, Yunkun Yang, Hongxi Zhou, Xianchao Liu, Rui Pan, He Yu, Jun Gou, Zhiming Wu, Jiang Wu, Faxian Xiu (修发贤), Yi Shi (施毅), Jun Wang (王军)

Sci China Mater, 2023, 66(4): 1484–1493



ARTICLE

Self-powered sensitive pressure sensor matrix based on patterned arrays of flexible (K,Na)NbO3 piezoelectric nanorods

基于图形化铌酸钾钠纳米棒阵列的自供电压力传感器

Lei Jiang, Mengrui Lu, Piaoyun Yang, Yijing Fan (范怡静), Hao Huang, Juan Xiong, Zhao Wang (王钊), Haoshuang Gu, John Wang

Sci China Mater, 2023, 66(4): 1494–1503



ARTICLE

Controlled synthesis of ultrathin metallic MoO2 nanosheets for van der Waals contact

超薄金属性MoO2纳米片可控合成及其范德华接触应用研究

Lizhen Fang, Huawei Liu, Wen Guan, Biyuan Zheng, Jieyuan Liang, Tinghao Wang, Xiaoli Zhu, Siyu Li, Dong Li (李东), Anlian Pan (潘安练) 

Sci China Mater, 2023, 66(4): 1504–1510



ARTICLE

Impact of surface free energy on two-dimensional crystallization

表面自由能对二维结晶的影响

Jiarong Yao, Lingjie Sun, Yanling Xiao, Jinyu Liu, Jiansheng Jie, Xuying Liu, Fangxu Yang, Yajing Sun, Rongjin Li (李荣金), Wenping Hu 

Sci China Mater, 2023, 66(4): 1511–1517



ARTICLE

Liquid crystal-like active layer for high-performance organic field-effect transistors

类液晶作为高性能有机场效应晶体管的有源层

Zhifang Wang, Daniel Martin-Jimenez, Yingying Zhang, Miguel Wiche, Lacheng Liu, Daniel Ebeling, Qigang Zhong, Florian Fontein, Andre Schirmeisen, Lizhen Huang, Zi Wang (王滋), Wenchong Wang (王文冲), Lifeng Chi (迟力峰)

Sci China Mater, 2023, 66(4): 1518–1526



ARTICLE

Articular cartilage-inspired 3D superelastic and fatigue-resistant spongy conductors against harsh environments

受关节软骨启发的耐疲劳和耐苛刻环境的三维超弹海绵导体

Tianyi Zhu, Qichun Feng, Kening Wan, Chao Zhang (张超), Bin Li, Tianxi Liu (刘天西)

Sci China Mater, 2023, 66(4): 1527–1538



ARTICLE

An ultra-tough and super-stretchable ionogel with multi functions towards flexible iontronics

一种面向柔性离子电子学的超强韧、可拉伸的多功能离子凝胶

Weiqing Zhan, Haoqi Zhang, Xiaolin Lyu (吕晓林), Zhong-Zhen Luo (罗中箴), Yan Yu, Zhigang Zou

Sci China Mater, 2023, 66(4): 1539–1550



ARTICLE

Design of all-phase-change-memory spiking neural network enabled by Ge-Ga-Sb compound

基于Ge-Ga-Sb介质的全相变脉冲神经网络的设计

Jun Lin, Xianliang Mai, Dayou Zhang, Kuan Wang, Huan Wang, Yi Li, Hao Tong, Yuhui He, Ming Xu, Xiangshui Miao

Sci China Mater, 2023, 66(4): 1551–1558



ARTICLE

Bio-synapse behavior controlled by interface engineering in ferroelectric tunnel memristors

利用界面工程来调控铁电隧道忆阻器的生物突触行为

Jianhui Zhao, Tianqi Yu, Yiduo Shao, Rui Guo (郭瑞), Weinan Lin, Gongjie Liu, Zhenyu Zhou, YiFei Pei, Jingjuan Wang, Kaixuan Sun, Xiaobing Yan (闫小兵), Jingsheng Chen (陈景升) 

Sci China Mater, 2023, 66(4): 1559–1568



ARTICLE

Biodegradable and flexible artificial nociceptor based on Mg/MgO threshold switching memristor

基于Mg/MgO阈值转变忆阻器的柔性生物可降解人工伤害感受器

Yaxiong Cao, Saisai Wang, Rui Wang, Yuhan Xin, Yaqian Peng, Jing Sun, Mei Yang, Xiaohua Ma, Ling Lv (吕玲), Hong Wang (王宏), Yue Hao

Sci China Mater, 2023, 66(4): 1569–1577



ARTICLE

Extreme environment-bearable polyimide film with a three-dimensional Ag microfiber conductive network for ultrahigh electromagnetic interference shielding

基于银微米纤维导电网络的超高电磁屏蔽且耐极端环境聚酰亚胺薄膜

Kangkang Zou, He Sun, Xueying Li, Shuangqin Yi, Jie Li, Zisong Zhou, Haolun Wang (王浩伦), Ding-Xiang Yan (鄢定祥)

Sci China Mater, 2023, 66(4): 1578–1586



ARTICLE

Core-shell LaOCl/LaFeO3 nanofibers with matched impedance for high-efficiency electromagnetic wave absorption

核壳结构LaOCl/LaFeO3纳米纤维的阻抗匹配设计及其电磁吸波性能研究

Yan Xing, Yicun Fan, Zhikai Yan, Biao Zhao (赵彪), Yujia Huang, Wei Pan (潘伟)

Sci China Mater, 2023, 66(4): 1587–1596



ARTICLE

Ultrafine cellulose nanocrystal-reinforced MXene biomimetic composites for multifunctional electromagnetic interference shielding

超细纤维素纳米晶增强MXene仿生复合材料的多功能电磁屏蔽性能

Na Wu, Bin Li, Fei Pan, Runa Zhang, Jiurong Liu (刘久荣), Zhihui Zeng (曾志辉)

Sci China Mater, 2023, 66(4): 1597–1606



ARTICLE

Self-cleaning solar water evaporation device based on polyaniline/TiO2/natural cellulose fibers for contaminant water

基于聚苯胺/二氧化钛/天然纤维素的污水自清洁太阳能水蒸发装置

Wenning Liu, Pengfei Li, Xiangqin Li, Yaqian He, Li An, Dan Qu, Xiayan Wang, Zaicheng Sun (孙再成)

Sci China Mater, 2023, 66(4): 1607–1614



ARTICLE

Mechanically excited thermometry in erbium ions

基于Er3+的力致温度传感

Leipeng Li, Jingjing Ning, Chongyang Cai, Zheng Zhu, Yixiao Han, Yuantian Zheng, Dengfeng Peng (彭登峰), Jianrong Qiu (邱建荣), Yanmin Yang (杨艳民)

Sci China Mater, 2023, 66(4): 1615–1622



ARTICLE

Fabrication of anti-counterfeiting patterns with angle-dependent colors by silkscreen printing and UV-curable photonic crystal inks

基于丝网印刷和光固化油墨制备具有角度变色效应的光子晶体防伪图案

Jieqiu Wang, Fei Pang, Qianqian Fu, Jianping Ge (葛建平)

Sci China Mater, 2023, 66(4): 1623–1631



ARTICLE

Interfacial charge mismatch enhanced energetic crystals for efficient energy-release and improved safety

界面电荷错配增强含能晶体高效能量释放及安全性

Yanzhou Qu, Menghua Zhang, Gang Li, Xinru Yang, Shaocong Deng, Feiyan Gong, Xu Zhao (赵煦), Zhijian Yang (杨志剑)

Sci China Mater, 2023, 66(4): 1632–1640


ARTICLE

Periodate-based molecular perovskites as promising energetic biocidal agents

高碘酸根分子钙钛矿作为新型含能杀菌剂

Zhi-Hong Yu, De-Xuan Liu, Yu-Yi Ling, Xiao-Xian Chen, Yu Shang, Shao-Li Chen, Zi-Ming Ye, Wei-Xiong Zhang (张伟雄), Xiao-Ming Chen

Sci China Mater, 2023, 66(4): 1641–1648



ARTICLE

Back stress dynamic balancing strategy enabled strength-ductility synergy in heterostructured Al-SiC composites

背应力平衡策略实现非均质Al-SiC复合材料的强塑性协同

Dongxin Mao, Xiangchen Meng, Yuming Xie, Yuexin Chang, Zhiwei Qin, Shuangming Xu, Long Wan, Yongxian Huang (黄永宪)

Sci China Mater, 2023, 66(4): 1649–1658



ARTICLE

Flexible fluorescent metal-organic frameworks towards highly stable optical fibers and biocompatible cell platforms

面向高稳定的光纤和生物相容性细胞平台的柔性荧光金属有机框架

Yue Yin, Hongbin Chen, Pengcheng Lin (林鹏程), Weitai Yu, Xiaobao Cao (曹小宝), Xinxin Sheng, Josep Puigmartí-Luis

Sci China Mater, 2023, 66(4): 1659–1669



LETTER

Achieving layered stacking within acyclic compounds through a tenon-and-mortise strategy

通过榫卯结构策略实现非环状化合物的层状排布

Baojing Tian, Qi Sun (孙琦), Ning Ding, Zhiyi Jiang, Shenghua Li (李生华)Siping Pang (庞思平)

Sci China Mater, 2023, 66(4): 1670–1674



LETTER

Significant tensile elasticity of nanoscale boron arsenide

纳米尺度砷化硼的超大拉伸弹性

Penghui Li, Xiaokuan Hao, Shenglin Lu, Linyan Wang, Guoyu Xiong, Ke Tong, Yu Duan, Yeqiang Bu, Guoying Gao (高国英), Hongtao Wang, Bo Xu, Anmin Nie (聂安民), Fei Tian (田非)

Sci China Mater, 2023, 66(4): 1675–1680


2023年文章目录(点击链接可查看各期目录)

《中国科学:材料科学》2023年第3期《中国科学:材料科学》2023年第2期《中国科学:材料科学》2023年第1期
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